Chloé Louise Booyens embarked on her television journey with a notable appearance in Whirlpool, a production that marked the beginning of her illustrious career in the small screen. The talented actress soon transitioned to the West End stage, making her professional debut in the Olivier Award-nominated Agatha Christie's Witness for the Prosecution, a critically acclaimed production that showcased her remarkable acting prowess from 2018 to 2019. Her film debut arrived in the form of The Art of War, a project that further solidified her position as a rising star in the entertainment industry.
Booyens' impressive resume continued to grow as she appeared in the multi-award-winning Olhouser in 2018, a testament to her exceptional acting abilities. The same year, she made significant contributions to several notable projects, including BBC 4's Searching for Cowardice, Tim Follin's At Dead Of Night, and the Bollywood film Jawaani Jaaneman.
In 2021, Booyens lent her voice to a soldier in Matthew Vaughn's period spy action comedy film The King's Man, a project that highlighted her impressive vocal range. Her lead role as Olivia in Vasyl Moskalenko's The Chernobyl Fallout, a production by Hollywood Ukraine, showcased her remarkable acting abilities and versatility as an actress.